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Liaquat Ali was a passenger on the bus and died at the scene.
Lorry driver William Mapstone died in hospital.
Insp John Thompson from Central Motorway Police Group Appeals said they would like to hear from anyone with information.
The man, who is not being named at this time, died in hospital just after 9pm last night. He was 65 and from Somerset. His family had travelled from their home in the Southwest to attend hospital. A third man remains in a critical condition in hospital. He was a passenger on the bus.
Latest ITV News reports
A bus driver who broke down on the M5 has today been sent to prison after failing a breath test. A lorry driver and bus passenger died.
West Midlands Police are continuing to investigate a collision on the M5 in the West Midlands.