CCTV footage from cameras linked to the RAF Club in Piccadilly opposite the Bomber Command memorial shows a man approaching it between 3.10am and 3.20am on Monday.
The new images released shows a man suspected of being responsible for the graffiti-desecration of the £7.5 million Bomber Command memorial.
More top news
Police are appealing for witnesses after a crash involving a car and three pedestrians in Islington.
Five rugby league legends were immortalised in bronze today outside Wembley Stadium.
Four people have been bailed after a three-year-old girl was shot in the stomach with an air riffle while she played in a park.